CCL:G: G09: Convergence Issues for H-Bonded Systems



Dear Sam ,

 Once i solved the problem of negative frequencies by subtracting or adding the coordinates of negative frequency (Get it > from freq. calculation) to the molecular specification coordinates (it should be the final coordinates in which negative frequency exist). If its painful then use matlab or any matrix adding/subtracting program to make the addition or subtraction easy. Hope it may work for you. By doing this we are mainly working against the negative frequency. hopefully you are using the keyword "nosymm" along with all others. 




Thanks & regards;

 ABHISHEK SHAHI

Research Scholar
Inorganic and Physical Chemistry
Indian Institute Of Science
Bangalore-12

India
E-mail:                  shahi#%#ipc.iisc.ernet.in
                                shahi.abhishek1984#%#gmail.com




On Thu, Sep 22, 2011 at 10:59 PM, Arne Dieckmann adieckma^googlemail.com <owner-chemistry#%#ccl.net> wrote:

Sent to CCL by: Arne Dieckmann [adieckma . googlemail.com]
I would not consider -1.9 wavenumbers an imaginary frequency. Have a look at the Gaussian manual and whitepapers, there is a section about this issue.

Cheers,
Arne

On Sep 22, 2011, at 8:25 AM, Sam Abrash sabrash]_[richmond.edu wrote:

>
> Sent to CCL by: "Sam   Abrash" [sabrash_+_richmond.edu]
> Hi Folks,
>
> I have a job involving hydrogen bonding of 3 acetylenes to the benzene cation.  I'm having trouble with the geometric convergence.  I was able to get the system to converge with normal convergence criteria, opt=calcall, and MaxStep=5, but then I got an imaginary frequency of -1.9 wavenumbers.
>
> Subsequently, I changed to Opt=tight, tried both calcfc and calcall, and have steadily reduced MaxStep to 1, but it still won't converge.  The force constant criteria have been met, but the problem is the displacement criteria.  Both this observation and looking at the structures with JMOL show that the problem is finding the minimum in a very shallow potential.
>
> Two questions.  First, is the 1.9 wavenumber imaginary frequency real or an artifact?  Second, any advice on how to force the system to converge?  Model chemistry is M062X/6-311++G**.
>
> Thanks!
> Sam>
>



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